The top carapace/shell does indeed resemble Tyranid armour. When I first saw these guys I too thought about their potential as a Tyranid conversion.
A head swap would indeed be in order as well as some filing and
GS to smooth out the boils and blisters and to steer the model away from its Nurglyness.
I'd also consider replacing the limbs with Tyranid ones but the present limbs could still work.
And for bonus points, a couple of well placed Tyranid carapace bits, perhaps on the abdomen.
Anyway... that's my vision for them