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As far as I can tell, they seem a lot more fractious and less structured than the loyalist chapters. They serve Chaos, after all. But I assume it also varies by individual legion: their mentality, how much of their strength survived the Horus Heresy and the ensuing Long War, whether they still have a Primarch whose leadership is beyond challenge, etc.
I get the sense that, without a Black Crusade to force them to get their ducks in a row, some legions effectively exist more as a shared legacy and martial philosophy than a proper organization. The Night Lords lost their Primarch, and I wouldn't be able to tell you who's their head honcho now without looking it up. The World Eaters are nominally led by Angron, but he doesn't strike me as the micromanaging type.
The Thousand Sons are probably fairly cohesive: they still have a Primarch (one of the more intelligent and proactive ones, too), and most of them are mindless automatons anyway. I'm guessing the Iron Warriors also have a formal chain of command, because it makes things Efficient. Not sure about the Alpha Legion... They're duplicitous, but they also seem very akin to a hive mind ("I am Alpharius").
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