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Hi I just got into 40k, and have brought the Dark Vengeance starter set. I want to add a Predator tank to my Dark Angel forces, do I just buy a normal space marines one and paint it green?

That is exactly what you do.

Barring any kind of specific Chapter associated livery(here, here, and here), the Predator for the Dark Angels is the stock Predator kit.

The Forge World stuff I linked is optional, not required. Some very similar stuff is included in the Ravenwing/Dark Angels Battleforce.

Indeed you do, I found the Chapter Upgrade frame that comes inside the Ravenwing Battalion to be useful for 'Dark Angeling' it up a little with iconography and bits of bling. Also reccomend using some magnets to make the weapons and options interchangable