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In general, Nyss Hunters tend to beat out Croe's for most lists: Nyss are a stronger generalist unit, and while Croe's has a higher theoretical damage output against living targets they typically need help from warcasters that can give them the backstrike opening they need (e.g. Scaverous). You could swap your current reinforcements with the Cutthroats though, since coming in from the side will give them the chance at backstrikes they usually don't get when having to charge in from the front.
As a general purchase I would probably do Nyss first, though.
EDIT: As for the rest of the list itself, I'm not so sure on the min+UA Bane Thralls: I feel like if you're going to commit to a UA, you want to put it on a full strength unit (since the UA costs the same regardless of size, you get more bang for your buck on a full unit). Also feels a bit odd to have two units of Banes and no Tartarus, although you could potentially work around that with feat to stall the enemy while your Banes get into position.
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