pushmould and greenstuff maybe.
If I was going to try and sculpt something similar, I'd use a fairly thick wire as a base (garden stores tend to have options), making the basic shape, then wrap greenstuff around it, and use silicone shaping tools to sculpt that into shape.
Might also be worth looking at eBay and bits sites for Mortis Engine spares - all the banshee stuff isn't used when build the Coven Throne option, so some must be going spare.
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