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If going for urban I would dial down the colours of the Captain. No point being Urban Camo, only to have a neon pastel/ psycadelic thing going on.
You can have startling effects with subtle colour schemes.
What I would say is that have 2 major things going for you.
1. A good colour scheme on your Tactical troops.
2. A very good level of brush control, this is a very good neat base coat.
If you want to improve the look then highlighting and Washes need to be applied. I would recommend dry brushing a light shade of of the Green/ Grey. Then use a Black, Devlin mud or Ogryn Flesh wash to bring it all together.
I think these will look amazing, if you highlight and wash these. The Wash will dull down the colours on the captains chest too.
EDIT - I always try to do keep all the same things on the model the same colours. So all the skulls in bone or white or whatever you've mixed them up a bit which is okay if you like it that way. However having little details like that helps tie the whole model together.
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