I wouldn't say Chaos is freedom, it might allow you to do acts that you wouldn't be able to do usually, but those acts are because you are required by your patron(s) to do so.
If your seen to not be taking skulls, Khorne will send one of his minions to turn yours into its new piss bucket.
On whether or not it's good, it all depends on how it gets used I guess. Laeran has been pointed out as a Chaos culture that seemed to have thrived, you could say the same for Nurth, Davin, 63:19, Chaos worlds that were cool beans before the Imperium came a knocking. So I guess it could be good. Or you have what happens when Chaos gets angry.
A good character to use as a point of reference would be Quixos from the Eisenhorn series. Wanted to use Chaos against Chaos but it eventually led to him falling.
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