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For me its Mechanicum Standard Grey.
Which is a shame, because its the base coat of all my army.... I just find it a bit soul destroying, undercoat the models and then base coat them..... and then they look EXACTLY like they did before I undercoated them

In order:
Black
White
Yellow

White is the bane of my existence. I first wanted to do a Raven Guard army when I first started, but after miserably painting a squad of Tac Marines and subsequently throwing them out due to having globs of paint from trying to layer white (this was back in 2001 when I wasn't aware of the existence of Simple Green), I put a kibosh on that idea.

I can paint white a bit better now, but I'm still not a fan of it. Yellow's not too fun either, but I've never really had that much of a problem with black.